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On March 31, 2007, the accused waylaid a man on a motorcycle with a machete and robbed him of his money, phone and a gold ring.
Sinaj has been involved in several cases of mobile phone theft and stealing valuables from cars after smashing the window glass.
The deceased were identified as Sivan Nair, a Siddha doctor, and his wife Prasannakumari.
The accused was taken into custody while on his way home from the airport.
The accused Madhusoothanan stole four sovereigns of gold and Rs 25,000 cash.
The missing gold is estimated to be worth more than Rs 2 crore.
The passengers filed a complaint with the Dharmapuri police station and Salem Railway Police in Tamil Nadu on Tuesday.
The theives had broken the window of the vehicle to get hold of the cash.
The failed attempted at the ATM in Valakom was caught on CCTV.