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Real Madrid earned a scrappy 1-0 victory at Sevilla, thanks to an own goal from keeper Bono, to ease the pressure on coach Zinedine Zidane.
Ousmane Dembele struck early and Lionel Messi converted a late penalty as Barcelona won 2-0 at Juventus after Alvaro Morata had three goals disallowed for offside for the Serie A side.
Villarreal defender Pau Torres scored an own goal right at the end of the first half to heap more pain on Unai Emery's side.
Cristiano Ronaldo scored a brace, including an unstoppable long-range goal, to give Juventus a 2-1 win over Olympique Lyonnais but it was not enough as the French side reached the quarterfinals on away goals.
Ronaldo broke the deadlock in first-half stoppage time with his 31st league goal of the season and Federico Bernardeschi added the second as Juve beat Sampdoria 2-0.
Having taken two points from their last three games, Juventus are on 77 points, seven ahead of Atalanta, who thumped Brescia 6-2 on Tuesday, with five matches remaining.
Arthur will remain at the Camp Nou until the end of the 2019-20 season, which has been extended until August because of the novel coronavirus pandemic, before moving to Turin.
The Turin club wrapped up an eighth successive league title last weekend but found themselves behind early on to a wonder-strike from Inter midfielder Radja Nainggolan.
Teenage striker Moise Kean struck again to give Juventus a late 2-1 win over AC Milan after their opponents had taken the lead and dominated most of the match on Saturday.
It looked a harsh decision as German referee Felix Brych reached for his red card after Ronaldo's seemingly innocuous tangle with Valencia defender Jeison Murillo in the area as Juve launched an attack down the left.