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The 28-year-old centre-back had his contract with HNK Sibenik terminated mutually.
Mohun Bagan's David Williams scored for the team but Javier Siverio's late strike ensured Hyderabad FC moved to the top of the table after a rip-roaring encounter.
Defender Juan Bernat, back-up goalkeeper Sergio Rico and midfielder Nathan Bitumazala were the other players who returned positive tests.
Liston Colaco and Roy Krishna scored for Bagan while Jorge Ortiz gave a late consolation for Goa.
Hugo Boumous scored a brace as ATKMB won 3-2.
Assistant coach Clifford Miranda will be the interim manager.
Santana became world No. 1 in 1966, the same year that he won Wimbledon.
It was the second consecutive victory for the Gaurs in a match that saw two red cards and eight yellow cards.
Atletico won 3-1 at Porto in a tense, ill-tempered game as both sides finished with 10 men.
SC East Begal are the lone team yet to win a match this season.