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"Congratulations to Arsenal. We were not good enough today," Klopp said. "It just shows the boys are human beings."
Liverpool moved five points clear atop the Premier League to set up a potential thriller on Sunday against third-placed Arsenal.
The German joined Liverpool in October, 2015, and has won the Champions League, Premier League, Club World Cup, FA Cup, League Cup and Super Cup, as well as the Community Shield during his time in charge.
Uruguayan Nunez put the seal on a dominant Liverpool display with his second goal in stoppage time.
The 31-year-old Salah, who has 151 Premier League goals for Liverpool, changed his boots at halftime and the switch paid off handsomely.
Manchester City slipped out of the top four as Tottenham Hotspur made up ground with a third consecutive victory, beating Everton 2-1 at home.
Diogo Dalot was sent off in stoppage time for two yellow cards -- both for dissent.
Leon Bailey's deflected strike after a surging run in the 74th minute sealed Villa's club record-equalling 14th successive home league win as they moved above City into third place.
Ten-man Chelsea beat Brighton & Hove Albion 3-2 at Stamford Bridge while fourth-placed Aston Villa needed a late Ollie Watkins goal to scrape a 2-2 draw at Bournemouth.
Trent Alexander-Arnold drilled in an 80th-minute equaliser with his right foot to deny City a 24th successive home win in all competitions.