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Kerala have 14 points from six games and are out of contention for a place in the quarterfinals.
The hosts, who gained a huge first innings lead of 183, declared their second innings on 265/6.
This was the 37-year-old's 29th five-wicket haul at the first-class level.
The 35-year-old also went past the tally of 5,000 first-class runs during the course of his knock.
Kerala have just eight points from five matches and their hopes of qualifying for the quarterfinals are almost over.
The hosts were bowled out for 312 shortly before tea, handing Kerala a lead of 38 runs. Kerala finished on 69/2 at close of play, extending the lead to 107.
The hosts were struggling at 100/4 in reply to Kerala's first innings total of 350.
Kerala fought back to reach 219/4 on the opening day of their Elite Group B match against Chhattisgarh.
Captain Rohan Kunnummal (37) and his opening partner Anand Krishan (12) were the batters dismissed. Sachin Baby (6) and Akshay Chandran (2) were at the crease. Kerala still trail the hosts by 88 runs going into the final day.
The home side finished the second day on 270/5 in reply to Kerala's first innings total of 227.