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Gokulam scored a 4-1 win in the I-League in New Delhi.
The defending champions lost 0-1 while TRAU climbed to fourth with the win.
Gokulam remain in third spot with 33 points from 19 games.
Farshad Noor scored the solitary goal in Vasco da Gama.
Gokulam jumped to third place with 27 points from 17 matches.
The match ended 2-1 in favour of the Kolkata side leaving Gokulam fourth in the table.
The win helped Punjab tie with Sreenidi Deccan on points (34) at the top of the table. Deccan are ahead on goal difference.
The defeat meant Gokulam could not capitalise on RoundGlass Punjab FC dropping points after conceding a last-minute equaliser to bottom-placed Sudeva Delhi.
Gokulam were reduced to 10 men in the 56th as Rahul Raju was sent off.
Thahir Zaman put the defending champions ahead in the 35th minute, while new recruit Jobby Justin doubled the lead in the 86th to make sure of three points.
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