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The accused Madhusoothanan stole four sovereigns of gold and Rs 25,000 cash.
The missing gold is estimated to be worth more than Rs 2 crore.
The passengers filed a complaint with the Dharmapuri police station and Salem Railway Police in Tamil Nadu on Tuesday.
The theives had broken the window of the vehicle to get hold of the cash.
The failed attempted at the ATM in Valakom was caught on CCTV.
The incident happened on January 30 on the Sulthan Bathery-Koliyadi road.
Sreedharan is notorious for ambushing transporters of hawala money on highways and robbing them of the cash.
The girl, a student of Kottarakkara Govt. High School was on the way to tuition class during the time of the attack
According to police, George was strangled to death during a robbery bid.
A special investigation team, led by Ajith V, District Superintendent of Police (SP), and that including two DySPs, has been formed to probe the broad daylight murder.